Terahertz nanoscopy of quantum-geometric photovoltaics in bilayer graphene

Abstract

The bulk photovoltaic effect (BPVE) provides a direct link between quantum geometry and nonlinear light-matter interactions, yet conventional far-field measurements cannot disentangle BPVE from contact- and interface-induced photothermoelectric signals. Here we develop cryogenic, polarization-sensitive terahertz microscopy with deep-subwavelength resolution and apply it to dual-gated AB bilayer graphene. Near resonance between the band gap and terahertz photon energy, we observe enhanced optical conductivity and spatially resolved BPVE. Polarization-dependent measurements reveal a characteristic twofold angular symmetry and a distinct shift-vector direction, both governed by crystalline symmetries and quantum geometry. The evolution of BPVE with carrier density and temperature provides a sensitive probe of the fine electronic structure of bilayer graphene, revealing signatures of trigonal warping and electron-hole asymmetry. Agreement with theory demonstrates that the terahertz nanoscopy of BPVE established here offers an optical lens into the interplay between band and quantum geometry in quantum materials.