Cooperative Shunt Photocatalysis of Pt Single Atoms and Nanoparticles for Efficient Methanol Conversion to Hydrogen and Formaldehyde.
Photocatalytic methanol dehydrogenation requires not only charge separation but, more critically, synchronized and rapid consumption of photogenerated electrons and holes-an unmet challenge in conventional Pt-based photocatalysts. Here we report a photocatalytic platform in which Pt single atoms (Pt SA) and Pt nanopart...