Author

Yongchao Wang

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Open access Oct 2026

Engineering of Redox-Active Residues Enhances P450 Peroxygenase Performance.

Cytochrome P450 peroxygenases depend on the high-valent iron-oxo intermediate Compound I (Cpd I) to activate C-H bonds. However, the nonproductive oxidative damage caused by Cpd I compromises enzyme stability and limits catalytic efficiency. Here, we report a rational protein engineering strategy to address this bottle...

Zi-Han Wang, Ming-Ming Qin, Yong-Chao Wang et al. · Angewandte Chemie · 0 citations

Aug 2026

A Cytochrome P450 Enzyme-Catalyzed Acetyl Migration in Cyanogramide Biosynthesis.

It is demonstrated that the cytochrome P450 monooxygenase CyaI catalyzes an oxidation reaction through a zwitterionic intermediate and facilitates a subsequent unusual C→N acetyl migration, which triggers a spontaneous intramolecular cyclization to forge the imidazolidin-4-one ring during 1 biosynthesis.

Yi-Guang Zhu, Yongchao Wang, Li-Ping Zhang et al. · Angewandte Chemie · 0 citations