Biomimetic Hydrogen-Bond Network Engineering Regulates the Catalytic Microenvironment to Enhance Urea Electrooxidation and Selective N2 Generation
As a crucial anodic pathway, the urea oxidation reaction (UOR) holds immense potential for the purification of nitrogenous sewage as well as the energy-saving generation of hydrogen power. However, conventional nickel-based catalysts often trigger detrimental C–N bond cleavage of urea, yielding deleterious by-product...