Fluorinated Segments Engineering with Strongly Electron Withdrawing Effect in Quasi Solid State Electrolyte for Fast Charging and High Voltage Lithium Metal Batteries
Polyether electrolytes (PE) suffer from strong Li+–ether oxygen coordination and poor high voltage oxidative stability. Herein, we use in situ copolymerization to covalently graft the strongly electron-withdrawing −CF3 groups onto the backbone, synthesizing FPME, which delocalizes electron density around ether oxygen...