The dynamic chemistry of covalent boron-oxygen bonds has been extensively leveraged to construct cutting-edge dynamic covalent polymer networks (DCPNs) with self-healing, repairable, and reprocessable properties. However, the inherent poor water resistance of the resulting structural units, such as boronic esters or...
Fan Zhang, Hui Zhou, Tian-Jun Yue et al.· Macromolecules· 0 citations
Millions of tons of polymer waste are generated annually from branched polyethylene-based single-use packaging and agricultural films, constituting a pressing global environmental concern. Nonalternating carbonylative chain walking polymerization offers a promising strategy, whereas fundamentally constrained by the i...
Zhi-Hao Zhang, Ji-Ning Zhang, Shi-Yu Chen et al.· Journal of the American Chem...· 1 citation
Developing cost-effective and highly efficient Lewis pair (LP) systems represents a powerful strategy for achieving living/controlled polymerization of (meth)acrylates, enabling the synthesis of functional polar vinyl polymers with diverse structures and topologies. Herein, a new class of strong nucleophilic tetra-hy...
Isotactic poly(propylene oxide) (iPPO) is a semicrystalline polyether that has emerged as a high-strength, photodegradable material for marine applications. To improve the accessibility of iPPO, catalysts with higher activity and selectivity are required. Using rational catalyst design informed by computational insight...
Bai-Hao Ren, Bryce M Lipinski, L. S. Morris et al.· Journal of the American Chem...· 1 citation
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