Ligand Electronics and Metal‐Site Acidity Enable High‐Voltage MOF Electrolytes for Quasi‐Solid‐State Lithium‐Metal Batteries
Lithium‐metal batteries (LMBs) coupled with Ni‐rich cathodes offer high energy density for next‐generation energy storage. Their practical implementation, however, is limited by electrolyte oxidation and interfacial degradation under high voltage. Metal‐organic frameworks (MOFs) would regulate ion solvation and sta...