Terahertz two-dimensional coherent spectroscopy: unlocking coherent quantum intraband nonlinear dynamics
Quantum materials host a rich spectrum of low-energy collective excitations- phonons, magnons, plasmons, polaritons, and Higgs modes- that fundamentally govern their emergent properties, but remain inaccessible to conventional linear THz spectroscopy when nonlinear pathways overlap or non-perturbative dynamics emerge....