S. Vasilchenko

Model-free Reconstruction of Molecular Energy Levels by Broadband Kilohertz-accurate Cavity-enhanced Spectroscopy

Assigning the lines of high-resolution molecular spectra to quantum states requires a Hamiltonian model and substantial expert intervention, so the spectra of larger molecules accumulate vast numbers of unassigned lines. Here we show that molecular energy levels can instead be reconstructed directly from the raw, unass...