A Targeted Functional‐Group Integration Strategy for Modulating Wide‐Bandgap Perovskites Toward Efficient Silicon/Perovskite Tandem Photovoltaics
Wide‐bandgap (WBG) perovskites featuring 1.65–1.70 eV bandgaps are highly desirable light‐harvesting layers to construct high‐performance tandem photovoltaics. However, the complex multi‐component precursor system, especially the asymmetric nucleation of I‐rich and Br‐rich phases during film formation, often leads...