Author

Liu-Peng Zhao

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Open access Sep 2026

A binuclear copper enzyme platform for enantioconvergent radical (pseudo)halogenation

Despite their intriguing native metalloenzymology, naturally occurring copper enzymes remain largely underexploited for new-to-nature biocatalytic reactions. Herein, we report the systematic investigation and reprogramming of natural copper enzymes to catalyze unnatural free radical (pseudo)halogenation reaction in a h...

Xiao-Wang Chen, O. Adeyemo, He-Yu Chen et al. · bioRxiv · 0 citations

Jul 2026

Directed Evolution of Nonheme Fe Enzymes for Enantioselective and Regiodivergent 1,3- and 1,4-Nitrogen Migration: Biocatalytic Asymmetric Synthesis of Noncanonical α- and β-Amino Acids.

Biocatalyst-controlled regioselective C(sp)-H functionalization of carboxylic acid derivatives provides a powerful method for the synthesis of noncanonical α- and β-amino acids. Herein, we report a nonheme Fe enzyme-catalyzed, regiodivergent, and enantioselective nitrogen migration, enabled by directed evolution of 1-a...

Huichong Liu, Liu-Peng Zhao, Shijia Li et al. · Journal of the American Chem... · 0 citations