The confinement effect of nanochannels (<2 nm) dictates the gas–liquid distribution at solid–liquid interfaces, yet the effect of interfacial chemistry on their kinetic behaviors lacks insightful understanding. Particularly, the interfacial CO2 transport mechanism is critical for CO2 capture in hydrated environments. H...
Wan-Ting Xie, P. Maitarad, T. Rungrotmongkol et al.· JACS Au· 0 citations
Solution‐processable covalent organic frameworks (COFs) are crucial for advancing practical applications, yet traditional top‐down exfoliation into solvophilic nanosheets suffers from low efficiency and limited scalability. This study presents a large‐scale homogeneous crystallization strategy to constitute a famil...
Electrochemical CO2 reduction to value-added multi-carbon products is attractive, whereas the low-efficiency C─C coupling hinders the electrocatalytic selectivity and activity. Herein, we synthesize a polyphosphazene network with a precise supramolecular configuration of the neighboring dual catalytic centers by introd...