ABSTRACT The synthesis of pyrroles, fundamental nitrogen‐heterocyclic scaffolds in pharmaceuticals and materials science, remains a synthetic challenge, typically requiring pre‐functionalized precursors and multi‐step protocols. Here, we report an efficient cascade synthesis of N‐substituted pyrroles directly from bio‐...
Hai-Feng Qi, Germán López Robledo, Jiang-Li Duan et al.· Angewandte Chemie· 0 citations
Optimizing promoters is crucial for designing efficient catalysts for ammonia (NH3) synthesis under mild conditions. However, this endeavor is often hampered by a fundamental trade-off: weak metal-promoter interactions (MPI) lead to promoter segregation, while excessively strong ones block active sites, both diminishin...
Xiuyun Wang, Jia-Hao Yu, Kailin Su et al.· Angewandte Chemie· 0 citations
Photocatalytic oxygen reduction offers a sustainable, solar-driven route for the green synthesis of hydrogen peroxide (H2O2), however it suffers from limited efficiency due to rapid charge recombination and poor selectivity toward the two-electron reduction pathway. Herein, crystalline poly(heptazine) imide (PHI) and p...
Auttaphon Chachvalvutikul, Hai-Feng Qi, Ren-Jun Liu et al.· Journal of Materials Chemist...· 0 citations
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