Light- and pH-Gated Reversible Modulation of Peptide Coacervates via Noncovalent Integration of Spiropyran Photoswitches.
Peptide coacervates formed via liquid-liquid phase separation (LLPS) have emerged as versatile cell-like compartments for protocell studies and spatially confined catalysis. However, achieving remote, noninvasive modulation of their assembly‒disassembly lifecycle remains a key challenge. Here, we report a supramolecula...