Coupling the Spin State Switching and CO2 Adsorption Operating at Different Temperatures in a Breathing Metal-Organic Framework.
Gas-responsive magnetic response arising from spin-crossover (SCO) phenomena is rare yet highly attractive for molecular sensing and spintronics. However, it remains unclear how gas uptake influences SCO behaviour when the two phenomena occur in separate temperature regimes. Herein, we report a strong influence of CO2...