Alloy-Assisted Formation of Vanadium-Rich Thiophosphates with Enhanced Charge Transport and Glassy Magnetism
Vanadium-based thiophosphates in the MPQ3/M2P2Q6 family provide an unusual platform for coupling mixed-metal valence, metal vacancies, and 2D magnetism, but access to phase-pure multimetal solid solutions with verified chemical homogeneity remains limited. Here, we show that multication alloying provides a route to i...